A multi-disciplinary research program was recently completed, sponsored by NASA Marshall Space Flight Center, on the subject of aerocapture of spacecraft weighing up to 5 metric tons at Mars. Heavier spacecraft will require deployable drag area beyond the dimensional limits of current and planned launch fairings. This research focuses on the approach of lightweight inflatable decelerators constructed with thin films, using fiber reinforcement and having a temperature limitation of 500 C. Trajectory analysis defines trajectories for a range of low ballistic coefficients for which convective heat flux is compatible with the material set. Fluid-Structure Interaction (FSI) tools are expanded to include the rarified flow regime. Several non-symmetrical configurations are evaluated for their capability to develop lift as part of the necessary trajectory control strategy. Manufacturing technology is developed for 3-D stretch forming of polyimide films and for tailored fiber reinforcement of thin films. Finally, the mass of the decelerator is estimated and compared to the mass of a traditional rigid aeroshell.